Formation of redox-active self-assembled polyelectrolyte-surfactant complexes integrating glucose oxidase on electrodes: Influence of the self-assembly solvent on the signal generation
In this work the effects of the self-assembly solvent on the structure and electrochemical behavior of redox-active polyelectrolyte-surfactant complexes cast on electrode supports from aqueous and DMF solutions are presented. The complex studied is formed by complexation of osmium complex-modified p...
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| Otros Autores: | , , |
| Formato: | Capítulo de libro |
| Lenguaje: | Inglés |
| Publicado: |
Elsevier
2015
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| Acceso en línea: | Registro en Scopus DOI Handle Registro en la Biblioteca Digital |
| Aporte de: | Registro referencial: Solicitar el recurso aquí |
| LEADER | 15875caa a22014777a 4500 | ||
|---|---|---|---|
| 001 | PAPER-13215 | ||
| 003 | AR-BaUEN | ||
| 005 | 20241209083659.0 | ||
| 008 | 190411s2015 xx ||||fo|||| 00| 0 eng|d | ||
| 024 | 7 | |2 scopus |a 2-s2.0-84932608452 | |
| 024 | 7 | |2 cas |a dodecyl sulfate, 151-41-7; glucose, 50-99-7, 84778-64-3; glucose oxidase, 9001-37-0; osmium, 7440-04-2; Electrolytes; Glucose Oxidase; Surface-Active Agents | |
| 030 | |a BIOEF | ||
| 040 | |a Scopus |b spa |c AR-BaUEN |d AR-BaUEN | ||
| 100 | 1 | |a Cortez, M.L. | |
| 245 | 1 | 0 | |a Formation of redox-active self-assembled polyelectrolyte-surfactant complexes integrating glucose oxidase on electrodes: Influence of the self-assembly solvent on the signal generation |
| 260 | |b Elsevier |c 2015 | ||
| 270 | 1 | 0 | |m Azzaroni, O.; Instituto de Investigaciones Fisicoquímicas Teóricas y Aplicadas (INIFTA), Departamento de Química, Facultad de Ciencias Exactas, Universidad Nacional de La Plata, CONICET, CC 16 Suc. 4, Argentina |
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| 506 | |2 openaire |e Política editorial | ||
| 520 | 3 | |a In this work the effects of the self-assembly solvent on the structure and electrochemical behavior of redox-active polyelectrolyte-surfactant complexes cast on electrode supports from aqueous and DMF solutions are presented. The complex studied is formed by complexation of osmium complex-modified polyallylamine (OsPA) with dodecyl sulfate (DS) surfactants. The structure of the films was characterized by GISAXS, showing that films present a lamellar mesostructure. However, when they are exposed to humid environments, films cast from aqueous solutions (OsPA-DSaq) undergo a structural transition that ultimately leads to the disappearance of the mesostructural order. On the other hand, OsPA-DS films cast from DMF solutions (OsPA-DSorg) revealed no significant changes upon exposure to humid environments. Both types of films were exposed to glucose oxidase (GOx), showing similar adsorption characteristics. Notwithstanding these similarities in GOx and content, OsPA-DSaq films revealed a more sensitive bioelectrocatalytical response to glucose as compared to OsPA-DSorg films. © 2015 Elsevier B.V. |l eng | |
| 536 | |a Detalles de la financiación: Centro Interdisciplinario de Nanociencia y Nanotecnología | ||
| 536 | |a Detalles de la financiación: Universidad de Buenos Aires, X0513 | ||
| 536 | |a Detalles de la financiación: Laboratório Nacional de Luz Síncrotron, LNLS, XRD2-14358, XRD2-13391, XRD2-11639, SXS-11642 | ||
| 536 | |a Detalles de la financiación: Agencia Nacional de Promoción Científica y Tecnológica, PICT 2011-0406, PICT 2013-0905, PPL 2011-003, PICT 2010-2554 | ||
| 536 | |a Detalles de la financiación: Consejo Nacional de Investigaciones Científicas y Técnicas | ||
| 536 | |a Detalles de la financiación: Max-Planck-Gesellschaft | ||
| 536 | |a Detalles de la financiación: The authors acknowledge the financial support from Universidad de Buenos Aires ( X0513 ), ANPCyT ( PICT 2011-0406 , PICT 2010-2554 , PICT 2013-0905 , and PPL 2011-003 ), Centro Interdisciplinario de Nanociencia y Nanotecnología ( CINN-ANPCyT-Argentina ) and Max-Planck-Gesellschaft ( Max Planck Partner Group for Functional Supramolecular Bioconjugates, INIFTA/MPIP ). O.A. and M.C. gratefully acknowledge the Laboratório Nacional de Luz Síncrotron ( LNLS, Campinas — Brazil ) for financial support and granting access to synchrotron facilities (XRD2-13391; XRD2-11639, XRD2-14358 and SXS-11642). M.L.C. acknowledges CONICET for a postdoctoral fellowship. M.C., O.A. and F.B. are CONICET fellows. | ||
| 593 | |a INQUIMAE, Departamento de Química Inorgánica, Analítica y Química Física, Facultad de Ciencias Exactas y Naturales, Universidad de Buenos Aires, Ciudad Universitaria, Pabellón 2, Buenos Aires, C1428EHA, Argentina | ||
| 593 | |a Instituto de Investigaciones Fisicoquímicas Teóricas y Aplicadas (INIFTA), Departamento de Química, Facultad de Ciencias Exactas, Universidad Nacional de La Plata, CONICET, CC 16 Suc. 4, La Plata, 1900, Argentina | ||
| 690 | 1 | 0 | |a ELECTROCHEMICAL ELECTRODES |
| 690 | 1 | 0 | |a ELECTRODES |
| 690 | 1 | 0 | |a GLUCOSE |
| 690 | 1 | 0 | |a GLUCOSE SENSORS |
| 690 | 1 | 0 | |a POLYELECTROLYTES |
| 690 | 1 | 0 | |a REDOX REACTIONS |
| 690 | 1 | 0 | |a SELF ASSEMBLY |
| 690 | 1 | 0 | |a SURFACE ACTIVE AGENTS |
| 690 | 1 | 0 | |a ADSORPTION CHARACTERISTIC |
| 690 | 1 | 0 | |a ELECTROCHEMICAL BEHAVIORS |
| 690 | 1 | 0 | |a GLUCOSE OXIDASES (GOX) |
| 690 | 1 | 0 | |a HUMID ENVIRONMENT |
| 690 | 1 | 0 | |a MESOSTRUCTURAL ORDERING |
| 690 | 1 | 0 | |a POLYELECTROLYTE-SURFACTANT COMPLEXES |
| 690 | 1 | 0 | |a SIGNAL GENERATION |
| 690 | 1 | 0 | |a STRUCTURAL TRANSITIONS |
| 690 | 1 | 0 | |a GLUCOSE OXIDASE |
| 690 | 1 | 0 | |a DODECYL SULFATE |
| 690 | 1 | 0 | |a GLUCOSE |
| 690 | 1 | 0 | |a GLUCOSE OXIDASE |
| 690 | 1 | 0 | |a OSMIUM |
| 690 | 1 | 0 | |a POLYELECTROLYTE |
| 690 | 1 | 0 | |a SOLVENT |
| 690 | 1 | 0 | |a SURFACTANT |
| 690 | 1 | 0 | |a ELECTROLYTE |
| 690 | 1 | 0 | |a SURFACTANT |
| 690 | 1 | 0 | |a ADSORPTION |
| 690 | 1 | 0 | |a AQUEOUS SOLUTION |
| 690 | 1 | 0 | |a ARTICLE |
| 690 | 1 | 0 | |a CHEMICAL STRUCTURE |
| 690 | 1 | 0 | |a COMPLEX FORMATION |
| 690 | 1 | 0 | |a COMPOSITE MATERIAL |
| 690 | 1 | 0 | |a CONCENTRATION (PARAMETERS) |
| 690 | 1 | 0 | |a CONTACT ANGLE |
| 690 | 1 | 0 | |a ELECTROCHEMICAL ANALYSIS |
| 690 | 1 | 0 | |a ELECTRODE |
| 690 | 1 | 0 | |a ELECTRON TRANSPORT |
| 690 | 1 | 0 | |a EXPOSURE |
| 690 | 1 | 0 | |a GLUCOSE OXIDATION |
| 690 | 1 | 0 | |a SYNTHESIS |
| 690 | 1 | 0 | |a CHEMISTRY |
| 690 | 1 | 0 | |a ELECTRODE |
| 690 | 1 | 0 | |a OXIDATION REDUCTION REACTION |
| 690 | 1 | 0 | |a ELECTRODES |
| 690 | 1 | 0 | |a ELECTROLYTES |
| 690 | 1 | 0 | |a GLUCOSE OXIDASE |
| 690 | 1 | 0 | |a OXIDATION-REDUCTION |
| 690 | 1 | 0 | |a SURFACE-ACTIVE AGENTS |
| 700 | 1 | |a Ceolín, Marcelo Raúl | |
| 700 | 1 | |a Azzaroni, O. | |
| 700 | 1 | |a Battaglini, Fernando | |
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