Depth resolved nonlinear optical nanoscopy

An electromagnetic field forced to vary along a plane with a spatial scale d much smaller than its free space wavelength λ decays exponentially along its normal with a decay length ∼ d. This decay, similar to that of the wavefunction of tunneling electrons, has allowed the development of scanning ne...

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Detalles Bibliográficos
Autor principal: Mochán, W.L
Otros Autores: López-Bastidas, C., Maytorena, J.A, Mendoza, B.S, Brudny, Vera Leonor
Formato: Capítulo de libro
Lenguaje:Inglés
Publicado: 2003
Acceso en línea:Registro en Scopus
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Registro en la Biblioteca Digital
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100 1 |a Mochán, W.L. 
245 1 0 |a Depth resolved nonlinear optical nanoscopy 
260 |c 2003 
270 1 0 |m Mochán, W.L.; Centro de Ciencias Físicas, Univ. Nac. Auton. de Mex., Apartado Postal 48-3, 62251 Cuernavaca, Morelos, Mexico; email: mochan@fis.unam.mx 
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506 |2 openaire  |e Política editorial 
520 3 |a An electromagnetic field forced to vary along a plane with a spatial scale d much smaller than its free space wavelength λ decays exponentially along its normal with a decay length ∼ d. This decay, similar to that of the wavefunction of tunneling electrons, has allowed the development of scanning near-field optical microscopes (SNOMs), reminiscent of scanning tunneling and atomic force microscopes, which have been able to resolve structures in the nanometer scale. However, existing SNOMs are unable to determine the depth below the surface from which the optical signals arise due to the monotonic decay of the optical evanescent probe fields. In this paper we study the optical second harmonic generation (SHG) produced by mixing of the evanescent fields produced by a SNOM tip. We show that employing an appropriately spatially-patterned tip, a non-monotonic non-linear probing field may be produced which has a maximum at a given distance beyond the tip, yielding a novel microscopy which may attain depth resolution with nanometric lengthscales. We estimate the size of the optical signal and we compare it with that arising in the usual SHG-based surface spectroscopy of centrosymmetric materials. © 2003 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.  |l eng 
593 |a Centro de Ciencias Físicas, Univ. Nac. Auton. de Mex., Apartado Postal 48-3, 62251 Cuernavaca, Morelos, Mexico 
593 |a Ctro. Cie. de la Materia Condensada, Univ. Nac. Auton. de México, Apartado Postal 2681, Ensenada, Baja California 22800, Mexico 
593 |a Centro de Investigaciones en Optica, León, Guanajuato, Mexico 
593 |a Departamento de Física, Fac. de Ciencias Exactas y Naturales, Universidad de Buenos Aires, Ciudad Universitaria Pab. I, 1428 Buenos Aires, Argentina 
700 1 |a López-Bastidas, C. 
700 1 |a Maytorena, J.A. 
700 1 |a Mendoza, B.S. 
700 1 |a Brudny, Vera Leonor 
773 0 |d 2003  |g v. 240  |h pp. 527-536  |k n. 3  |p Phys. Status Solidi B Basic Res.  |x 03701972  |t Physica Status Solidi (B) Basic Research 
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