Reversible modulation of the redox activity in conducting polymer nanofilms induced by hydrophobic collapse of a surface-grafted polyelectrolyte

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We present the covalent modification of a Pani-like conducting polymer (polyaminobenzylamine, PABA) by grafting of a polyelectrolyte brush (poly [2-(methacryloyloxy)-ethyl-trimethylammonium chloride], PMETAC). As PABA has extra pendant amino moieties, the grafting procedure does not affect the backb...

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Autor principal: Fenoy, G.E
Otros Autores: Giussi, J.M, von Bilderling, C., Maza, E.M, Pietrasanta, L.I, Knoll, W., Marmisollé, W.A, Azzaroni, O.
Formato: Capítulo de libro
Lenguaje:Inglés
Publicado: Academic Press Inc. 2018
Acceso en línea:Registro en Scopus
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024 7 |2 scopus  |a 2-s2.0-85041846027 
024 7 |2 cas  |a nitrogen, 7727-37-9; perchlorate, 14797-73-0 
040 |a Scopus  |b spa  |c AR-BaUEN  |d AR-BaUEN 
030 |a JCISA 
100 1 |a Fenoy, G.E. 
245 1 0 |a Reversible modulation of the redox activity in conducting polymer nanofilms induced by hydrophobic collapse of a surface-grafted polyelectrolyte 
260 |b Academic Press Inc.  |c 2018 
270 1 0 |m Marmisollé, W.A.; Instituto de Investigaciones Fisicoquímicas Teóricas y Aplicadas (INIFTA), Departamento de Química – Facultad de Ciencias Exactas, Universidad Nacional de La Plata (UNLP), CONICET, 64 and 113, Argentina; email: wmarmi@inifta.unlp.edu.ar 
506 |2 openaire  |e Política editorial 
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520 3 |a We present the covalent modification of a Pani-like conducting polymer (polyaminobenzylamine, PABA) by grafting of a polyelectrolyte brush (poly [2-(methacryloyloxy)-ethyl-trimethylammonium chloride], PMETAC). As PABA has extra pendant amino moieties, the grafting procedure does not affect the backbone nitrogen atoms that are implicated in the electronic structure of the conducting polymers. Moreover, perchlorate anions interact very strongly with the quaternary ammonium pendant groups of PMETAC through ion pairing. Therefore, the grafting does not only keep the electroactivity of PABA in aqueous solutions but it adds the ion-actuation properties of the PMETAC brush to the modified electrode as demonstrated by contact angle measurements and electrochemical methods. In this way, the conjugation of the electron transfer properties of the conducting polymer with the anion responsiveness of the integrated brush renders perchlorate actuation of the electrochemical response. These results constitute a rational integration of nanometer-sized polymer building blocks that yields synergism of functionalities and illustrate the potentialities of nanoarchitectonics for pushing the limits of soft material science into the nanoworld. © 2018 Elsevier Inc.  |l eng 
536 |a Detalles de la financiación: 3911 
536 |a Detalles de la financiación: Austrian Institute of Technology 
536 |a Detalles de la financiación: Marie Curie Cancer Care 
536 |a Detalles de la financiación: Ashikaga Institute of Technology 
536 |a Detalles de la financiación: Universidad Nacional de La Plata, UNLP, PPID-X016 
536 |a Detalles de la financiación: Agencia Nacional de Promoción Científica y Tecnológica, PICT-2015-0346, PICT-2013-0905, PICT-2015-0239 
536 |a Detalles de la financiación: Consejo Nacional de Investigaciones Científicas y Técnicas, PIP 11220130100619CO 
536 |a Detalles de la financiación: 612704 
536 |a Detalles de la financiación: The authors acknowledge financial support from ANPCyT ( PICT-2013-0905 , PICT-2015-0239 , PICT-2015-0346 ), Universidad Nacional de La Plata ( PPID-X016 ), CONICET ( PIP 11220130100619CO ), the Austrian Institute of Technology GmbH (AIT–CONICET Partner Group: “Exploratory Research for Advanced Technologies in Supramolecular Materials Science” – Exp. 4947/11, Res. No. 3911, 28-12-2011) and the Marie Curie project “ Hierarchical functionalization and assembly of Graphene for multiple device fabrication ” ( HiGRAPHEN ) (Grant ref: 612704 ). JMG, CvB, EMM, LIP, WAM and OA are CONICET staff members. GEF gratefully acknowledges a Doctoral Scholarship from CONICET. 
593 |a Instituto de Investigaciones Fisicoquímicas Teóricas y Aplicadas (INIFTA), Departamento de Química – Facultad de Ciencias Exactas, Universidad Nacional de La Plata (UNLP), CONICET, 64 and 113, La Plata, 1900, Argentina 
593 |a Instituto de Investigación e Ingeniería Ambiental, Universidad Nacional de San Martín, 25 de Mayo y Francia, 1 piso (1650), Buenos Aires, Argentina 
593 |a Departamento de Física, Facultad de Ciencias Exactas y Naturales, Universidad de Buenos Aires, Buenos Aires, C1428EHA, Argentina 
593 |a Soft Matter Nanotechnology Group, CIC biomaGUNE, Paseo Miramón 182, San Sebastián, Gipuzkoa 20009, Spain 
593 |a Instituto de Física de Buenos Aires (IFIBA, UBA-CONICET), Facultad de Ciencias Exactas y Naturales, Universidad de Buenos Aires, Buenos Aires, C1428EHA, Argentina 
593 |a Centro de Microscopías Avanzadas Facultad de Ciencias Exactas y Naturales, Universidad de Buenos Aires, Buenos Aires, C1428EHA, Argentina 
593 |a Austrian Institute of Technology, Donau-City-Strasse 1, Vienna, 1220, Austria 
690 1 0 |a ANION RESPONSIVENESS 
690 1 0 |a CONDUCTING POLYMERS 
690 1 0 |a NANOARCHITECTONICS 
690 1 0 |a POLYANILINE 
690 1 0 |a POLYMER BRUSHES 
690 1 0 |a CHLORINE COMPOUNDS 
690 1 0 |a ELECTRONIC STRUCTURE 
690 1 0 |a GRAFTING (CHEMICAL) 
690 1 0 |a INORGANIC COMPOUNDS 
690 1 0 |a IONS 
690 1 0 |a NANOSCIENCE 
690 1 0 |a NEGATIVE IONS 
690 1 0 |a POLYANILINE 
690 1 0 |a POLYELECTROLYTES 
690 1 0 |a REDOX REACTIONS 
690 1 0 |a SOLUTIONS 
690 1 0 |a COVALENT MODIFICATIONS 
690 1 0 |a ELECTROCHEMICAL METHODS 
690 1 0 |a ELECTROCHEMICAL RESPONSE 
690 1 0 |a HYDROPHOBIC COLLAPSE 
690 1 0 |a NANOARCHITECTONICS 
690 1 0 |a POLYELECTROLYTE BRUSHES 
690 1 0 |a POLYMER BRUSHES 
690 1 0 |a POLYMER BUILDING BLOCKS 
690 1 0 |a CONDUCTING POLYMERS 
690 1 0 |a NANOFILM 
690 1 0 |a NITROGEN 
690 1 0 |a PERCHLORATE 
690 1 0 |a POLYAMINOBENZYLAMINE 
690 1 0 |a POLYELECTROLYTE 
690 1 0 |a POLYMER 
690 1 0 |a QUATERNARY AMMONIUM DERIVATIVE 
690 1 0 |a UNCLASSIFIED DRUG 
690 1 0 |a AQUEOUS SOLUTION 
690 1 0 |a ARTICLE 
690 1 0 |a CONTACT ANGLE 
690 1 0 |a ELECTROCHEMICAL ANALYSIS 
690 1 0 |a HYDROPHOBICITY 
690 1 0 |a MODULATION 
690 1 0 |a PRIORITY JOURNAL 
700 1 |a Giussi, J.M. 
700 1 |a von Bilderling, C. 
700 1 |a Maza, E.M. 
700 1 |a Pietrasanta, L.I. 
700 1 |a Knoll, W. 
700 1 |a Marmisollé, W.A. 
700 1 |a Azzaroni, O. 
773 0 |d Academic Press Inc., 2018  |g v. 518  |h pp. 92-101  |p J. Colloid Interface Sci.  |x 00219797  |w (AR-BaUEN)CENRE-15  |t Journal of Colloid and Interface Science 
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856 4 0 |u https://doi.org/10.1016/j.jcis.2018.02.014  |y DOI 
856 4 0 |u https://hdl.handle.net/20.500.12110/paper_00219797_v518_n_p92_Fenoy  |y Handle 
856 4 0 |u https://bibliotecadigital.exactas.uba.ar/collection/paper/document/paper_00219797_v518_n_p92_Fenoy  |y Registro en la Biblioteca Digital 
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962 |a info:eu-repo/semantics/article  |a info:ar-repo/semantics/artículo  |b info:eu-repo/semantics/publishedVersion 
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