Electronic, magnetic, and spectroscopic properties of binuclear diruthenium tetracarboxylates: A theoretical and experimental study

The electronic structure of binuclear diruthenium tetracarboxylates, in both the divalent Ru2II,II(O2CR)4 and the mixed-valent Ru2II,III(O2CR)4X (X = anion) states is studied by means of ZINDO/S-MRCI and DFT calculations. Both methods predict a (π*)2(δ*)2 ground-state configuration for the divalent...

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Detalles Bibliográficos
Autor principal: Estiú, G.
Otros Autores: Cukiernik, F.D, Maldivi, P., Poizat, O.
Formato: Capítulo de libro
Lenguaje:Inglés
Publicado: 1999
Acceso en línea:Registro en Scopus
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Registro en la Biblioteca Digital
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100 1 |a Estiú, G. 
245 1 0 |a Electronic, magnetic, and spectroscopic properties of binuclear diruthenium tetracarboxylates: A theoretical and experimental study 
260 |c 1999 
270 1 0 |m Estiú, G.; CEQUINOR, Departamento de Quimica, Univ. Nacional de la Plata, La Plata (1900), Argentina 
506 |2 openaire  |e Política editorial 
504 |a Stephenson, T.A., Wilkinson, G.J., (1966) J. Inorg. Nucl. Chem., 8, p. 2285 
504 |a Bennet, M.J., Caulton, K.G., Cotton, F.A., (1969) Inorg. Chem., 8, p. 1 
504 |a Aquino, M.A.S., (1998) Coord. Chem. Rev., 170, p. 141 
520 3 |a The electronic structure of binuclear diruthenium tetracarboxylates, in both the divalent Ru2II,II(O2CR)4 and the mixed-valent Ru2II,III(O2CR)4X (X = anion) states is studied by means of ZINDO/S-MRCI and DFT calculations. Both methods predict a (π*)2(δ*)2 ground-state configuration for the divalent species, contrary to the (π*)3(δ*)1 previously predicted by SCF-Xα calculations, but in agreement with magnetic measurements that show a strong Zero Field Splitting. © 1999 American Chemical Society.  |l eng 
593 |a CEQUINOR, Departamento de Quimica, Univ. Nacional de la Plata, La Plata (1900), Argentina 
593 |a INQUIMAE, Depto. Quim. Inorg., Analitica Q.F., Ciudad Universitaria, Núñez, 1428, Argentina 
593 |a Instituto de Ciencias, Univ. Nacional de General Sarmiento, Roca 850, 1663 San Miguel, Buenos Aires, Argentina 
593 |a Lab. de Chimie de Coordination, Serv. de Chim. Inorg. et Biologique, CEA/Grenoble, 17 Rue des Martyrs, 38054 Grenoble, France 
593 |a Lab. Spectrochimie Infrafouge Raman, CNRS, 2 Rue Henri Dunant, 94320 Thiais, France 
700 1 |a Cukiernik, F.D. 
700 1 |a Maldivi, P. 
700 1 |a Poizat, O. 
773 0 |d 1999  |g v. 38  |h pp. 3030-3039  |k n. 13  |p Inorg. Chem.  |x 00201669  |w (AR-BaUEN)CENRE-60  |t Inorganic Chemistry 
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