Dependence of the network structure of cured styrene butadiene rubber on the sulphur content

An investigation about the dependence of the physical properties of styrene-butadiene rubber copolymers (cured with different sulphur content, in order to obtain various networks) on the crosslink density was carried out by means of dynamical mechanical analysis, differential scanning calorimetry an...

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Autor principal: Salgueiro, Walter Alberto
Otros Autores: Marzocca, Angel José, Somoza, Alberto Horacio, Consolati, Gianni, Cerveny, S., Quasso, F., Goyanes, Silvia Nair
Formato: Capítulo de libro
Lenguaje:Inglés
Publicado: Elsevier Ltd 2004
Acceso en línea:Registro en Scopus
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LEADER 09075caa a22012737a 4500
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003 AR-BaUEN
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024 7 |2 scopus  |a 2-s2.0-3342881089 
024 7 |2 cas  |a 1,3 butadiene, 106-99-0, 25339-57-5; rubber, 9006-04-6; sulfur, 13981-57-2, 7704-34-9 
030 |a POLMA 
040 |a Scopus  |b spa  |c AR-BaUEN  |d AR-BaUEN 
100 1 |a Salgueiro, Walter Alberto 
245 1 0 |a Dependence of the network structure of cured styrene butadiene rubber on the sulphur content 
260 |b Elsevier Ltd  |c 2004 
270 1 0 |m Somoza, A.; IFIMAT-UNCentro, Pinto 399, B7000GHG, Tandil, Argentina; email: asomoza@exa.unicen.edu.ar 
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504 |a Deng, J.S., Isayev, I., (1991) Rubber Chem Technol, 64, p. 296 
504 |a Kirkegaard P, Pedersen NJ, Eldrup M. PATFIT Program Risø-M-2740 RNL; Roskilde, Denmark; 1989; Gronsky, W., Hoffman, U., Simon, G., Wutzler, A., Straube, E., (1992) Rubber Chem Technol, 65, p. 63 
504 |a Sircar, A.K., (1997) Thermal Characterization of Polymeric Materials, p. 980. , E.A. Turi. San Diego: Academic Press 
504 |a Ito, Y., Mohamed, H.F.M., Tanaka, K., Okamoto, K., Lee, K., (1996) J Radioanal Nucl Chem, Articles, 211, p. 211 
504 |a Bartos, J., Sausa, O., Kristiak, J., Blochowicz, T., Rossler, E., (2001) J Phys: Condens Matter, 13, p. 11473 
504 |a Wang, Y.Y., Nakanishi, H., Yean, Y.C., Sandreczki, T.C., (1990) J Polym Sci, Part B, Polym Phys, 28, p. 1431 
504 |a Wang, C.L., Hirade, T., Maurer, F.J.H., Eldrup, M., Pedersen, N.J., (1998) J Chem Phys, 108, p. 4654 
504 |a Srithawatpong, R., Peng, Z.L., Olson, B.G., Jamieson, A.M., Simha, R., McGerwey, J.D., Maier, T.R., Ishida, H., (1999) J Polym Sci, Part B, Polym Phys, 37, p. 2754 
504 |a Simha, R., Wilson, P.S., Olabisi, O., (1973) Kolloid-Z Z Polym, 251, p. 402 
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504 |a Jean, Y.C., Sandreczki, T.C., Ames, D.P., (1986) J Polym Sci, Part B: Polym Phys, 24, p. 1247 
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506 |2 openaire  |e Política editorial 
520 3 |a An investigation about the dependence of the physical properties of styrene-butadiene rubber copolymers (cured with different sulphur content, in order to obtain various networks) on the crosslink density was carried out by means of dynamical mechanical analysis, differential scanning calorimetry and positron annihilation lifetime spectroscopy. SBR specimens were cured with different sulphur content, in order to obtain various networks. On increasing the crosslink density, the glass transition temperature increases and the fractional free volume decreases. The thermal expansion coefficient of the free volume decreases in the rubbery phase by increasing the crosslink density, owing to the slower rate of expansion of nanoholes; furthermore, it seems influenced by the percentage of polysulfide density. The density of nanoholes is independent of the temperature, but decreases on adding sulphur. The results can be framed within the Simha-Somcynsky free volume theory. © 2004 Published by Elsevier Ltd.  |l eng 
536 |a Detalles de la financiación: Secretaría de Ciencia y Técnica, Universidad de Buenos Aires 
536 |a Detalles de la financiación: Universidad de Buenos Aires, UBACYT X-150 
536 |a Detalles de la financiación: Ministero dell’Istruzione, dell’Università e della Ricerca, MIUR 
536 |a Detalles de la financiación: Fundación Antorchas 
536 |a Detalles de la financiación: Consejo Nacional de Investigaciones Científicas y Técnicas, PIP N o 02825/01 
536 |a Detalles de la financiación: Universidad Nacional del Centro de la Provincia de Buenos Aires 
536 |a Detalles de la financiación: This work was supported by Consejo Nacional de Investigaciones Cientı́ficas y Técnicas (PIP N o 02825/01), Comisión de Investigaciones Cientı́ficas de la Provincia de Buenos Aires, Secretarı́a de Ciencia y Técnica (UNCentro), University of Buenos Aires (Project UBACYT X-150) and Fundación Antorchas, Argentina. G.C. acknowledges the support by the Ministero dell'Istruzione, dell'Università e della Ricerca through the MIUR-Cofin 2002 project (prot. n. 2002033184_005). O. Toscano and M.T. Maldonado are acknowledged by their technical assistance. 
593 |a IFIMAT-UNCentro, Pinto 399, B7000GHG, Tandil, Argentina 
593 |a Comn. Invest. Cie. Provincia B., Calle 526 e Loy 11, 1900 la Plata, B7000GHG, Tandil, Argentina 
593 |a LPMPyMC, Departamento de Física, Fac. Cie. Exact. Y Nat., Univ. N., Buenos Aires, Argentina 
593 |a Consejo Nac. Invest. Cie. Y T., Argentina 
593 |a Ist. Naz. Fis. Della Materia D., Politecnico di Milano, Piazza Leonardo Da Vinci 32, I-20133, Milano, Italy 
593 |a Inst. de Fisica de Materiales Tandil, Fisica, Pinto 399, 7000 Tandil, Argentina., Argentina 
690 1 0 |a FREE VOLUME 
690 1 0 |a NANOHOLE 
690 1 0 |a SBR COPOLYMER 
690 1 0 |a COPOLYMERS 
690 1 0 |a CROSSLINKING 
690 1 0 |a DIFFERENTIAL SCANNING CALORIMETRY 
690 1 0 |a GLASS TRANSITION 
690 1 0 |a POLYSULFIDES 
690 1 0 |a POSITRON ANNIHILATION SPECTROSCOPY 
690 1 0 |a DYNAMICAL MECHANICAL ANALYSIS 
690 1 0 |a NANOHOLES 
690 1 0 |a POSITRON ANNIHILATION LIFETIME SPECTROSCOPY 
690 1 0 |a STYRENE 
690 1 0 |a 1,3 BUTADIENE 
690 1 0 |a COPOLYMER 
690 1 0 |a RUBBER 
690 1 0 |a STYRENE DERIVATIVE 
690 1 0 |a SULFUR 
690 1 0 |a ARTICLE 
690 1 0 |a CHEMICAL ANALYSIS 
690 1 0 |a CHEMICAL STRUCTURE 
690 1 0 |a CROSS LINKING 
690 1 0 |a DENSITY 
690 1 0 |a DIFFERENTIAL SCANNING CALORIMETRY 
690 1 0 |a DYNAMICS 
690 1 0 |a GLASS TRANSITION TEMPERATURE 
690 1 0 |a POSITRON 
690 1 0 |a SPECTROSCOPY 
690 1 0 |a POLYMER SCIENCE 
700 1 |a Marzocca, Angel José 
700 1 |a Somoza, Alberto Horacio 
700 1 |a Consolati, Gianni 
700 1 |a Cerveny, S. 
700 1 |a Quasso, F. 
700 1 |a Goyanes, Silvia Nair 
773 0 |d Elsevier Ltd, 2004  |g v. 45  |h pp. 6037-6044  |k n. 17  |p Polymer  |x 00323861  |w (AR-BaUEN)CENRE-350  |t Polymer 
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856 4 0 |u https://doi.org/10.1016/j.polymer.2004.05.008  |y DOI 
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