Dynamics of adsorption of hydroxypropyl methylcellulose at the air-water interface

Surface dynamic properties (surface pressure and surface dilatational properties) of three commercial hydroxypropyl methylcellulose (HPMC) adsorbed at the air-water interface are presented in this paper as a function of adsorption time. Experiments were performed at constant temperature (20 °C), pH...

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Autor principal: Pérez, O.E
Otros Autores: Sánchez, C.C, Pilosof, A.M.R, Rodríguez Patino, J.M
Formato: Capítulo de libro
Lenguaje:Inglés
Publicado: 2008
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100 1 |a Pérez, O.E. 
245 1 0 |a Dynamics of adsorption of hydroxypropyl methylcellulose at the air-water interface 
260 |c 2008 
270 1 0 |m Rodríguez Patino, J.M.; Departamento de Ingeniería Química, Facultad de Química, Universidad de Sevilla, c/Prof. Garcia Gonzalez, 1, 41012 Sevilla, Spain; email: jmrodri@us.es 
506 |2 openaire  |e Política editorial 
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520 3 |a Surface dynamic properties (surface pressure and surface dilatational properties) of three commercial hydroxypropyl methylcellulose (HPMC) adsorbed at the air-water interface are presented in this paper as a function of adsorption time. Experiments were performed at constant temperature (20 °C), pH 7, and ionic strength 0.05 M. The dynamics of adsorption and the surface dilatational properties were measured simultaneously for different food-grade HPMC (called E4M, E50LV, and F4M), at bulk concentrations (CHPMC) ranging from 1×10-4 to 1% wt. It was found that the surface pressure (π) increased with the HPMC bulk concentration, which may be associated with HPMC adsorption. These phenomena have been related to HPMC diffusion to the interface (at short adsorption time) and to molecular interactions (at long-term adsorption). The HPMC films behaved as viscoelastic as deduced from the surface dilatational elasticity (Ed) and the loss angle tangent (Tan δ) evolution upon time. The values of Ed showed different behavior with the HPMC bulk concentration, which reflect structural differences in the adsorbed film. Differences in the dynamics of adsorption and surface dilatational properties between different HPMCs have been related to molecular differences, such as the molecular weight, degree of substitution, molar substitution, etc. © 2007 Elsevier Ltd. All rights reserved.  |l eng 
536 |a Detalles de la financiación: Consejo Nacional de Investigaciones Científicas y Técnicas 
536 |a Detalles de la financiación: Universidad de Buenos Aires 
536 |a Detalles de la financiación: Comisión Interministerial de Ciencia y Tecnología, AGL2004-1306/ALI 
536 |a Detalles de la financiación: Consejo Nacional de Investigaciones Científicas y Técnicas 
536 |a Detalles de la financiación: CYTED Ciencia y Tecnología para el Desarrollo, XI.17 
536 |a Detalles de la financiación: This research was supported by CYTED through project XI.17 and by CICYT through grant AGL2004-1306/ALI. The authors also acknowledge the support from Universidad de Buenos Aires, Agencia Nacional de Investigaciones Científicas y Técnicas, and Consejo Nacional de Investigaciones Científicas y Técnicas de la República Argentina. 
593 |a Departamento de Industrias, Facultad de Ciencias Exactas y Naturales, Universidad de Buenos Aires. Ciudad Universitaria, 1428 Buenos Aires, Argentina 
593 |a Departamento de Ingeniería Química, Facultad de Química, Universidad de Sevilla, c/Prof. Garcia Gonzalez, 1, 41012 Sevilla, Spain 
690 1 0 |a ADSORPTION 
690 1 0 |a AIR-WATER INTERFACE 
690 1 0 |a BIOPOLYMER 
690 1 0 |a BREWSTER ANGLE MICROSCOPY 
690 1 0 |a HYDROXYPROPYL METHYLCELLULOSE 
690 1 0 |a POLYSACCHARIDE 
690 1 0 |a SURFACE DILATATIONAL PROPERTIES 
690 1 0 |a SURFACE PRESSURE 
690 1 0 |a SURFACE RHEOLOGY 
700 1 |a Sánchez, C.C. 
700 1 |a Pilosof, A.M.R. 
700 1 |a Rodríguez Patino, J.M. 
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