QSPR modeling of Gibbs free energy of organic compounds by weighting of nearest neighboring codes

We examine the encoding of chemical structure of organic compounds by Labeled Hydrogen-Filled Graphs (LHFGs). Quantitative Structure-Property Relationships (QSPR) for a representative set of 150 organic molecules have been derived by means of the optimization of correlation weights of local invarian...

Descripción completa

Guardado en:
Detalles Bibliográficos
Autores principales: Castro, Eduardo Alberto, Toropova, Alla P., Toropov, Andrey A., Mukhamedjanova, D. V.
Formato: Articulo
Lenguaje:Inglés
Publicado: 2005
Materias:
Acceso en línea:http://sedici.unlp.edu.ar/handle/10915/133006
Aporte de:
id I19-R120-10915-133006
record_format dspace
institution Universidad Nacional de La Plata
institution_str I-19
repository_str R-120
collection SEDICI (UNLP)
language Inglés
topic Química
QSPR
Gibbs free energy
local invariant
nearest neighboring code
correlation weights
spellingShingle Química
QSPR
Gibbs free energy
local invariant
nearest neighboring code
correlation weights
Castro, Eduardo Alberto
Toropova, Alla P.
Toropov, Andrey A.
Mukhamedjanova, D. V.
QSPR modeling of Gibbs free energy of organic compounds by weighting of nearest neighboring codes
topic_facet Química
QSPR
Gibbs free energy
local invariant
nearest neighboring code
correlation weights
description We examine the encoding of chemical structure of organic compounds by Labeled Hydrogen-Filled Graphs (LHFGs). Quantitative Structure-Property Relationships (QSPR) for a representative set of 150 organic molecules have been derived by means of the optimization of correlation weights of local invariants of the LHFGs. We have tested as local invariants Morgan extended connectivity of zero- and first order, numbers of path of length 2 (P2) and valence shells of distance of 2 (S2) associated with each atom in the molecular structure, and the Nearest Neighboring Codes (NNC). The best statistical characteristics for the Gibbs free energy has been obtained for the NNC weighting. Statistical parameters corresponding to this model are the following <i>n</i> = 100, <i>r</i><sup>2</sup> = 0.9974, <i>s</i> = 5.136 kJ/mol, <i>F</i> = 38319 (training set); <i>n</i> = 50, <i>r</i><sup>2</sup> = 0.9990, <i>s</i> = 3.405 kJ/mol, <i>F</i> = 48717 (test set). Some possible further developments are pointed out.
format Articulo
Articulo
author Castro, Eduardo Alberto
Toropova, Alla P.
Toropov, Andrey A.
Mukhamedjanova, D. V.
author_facet Castro, Eduardo Alberto
Toropova, Alla P.
Toropov, Andrey A.
Mukhamedjanova, D. V.
author_sort Castro, Eduardo Alberto
title QSPR modeling of Gibbs free energy of organic compounds by weighting of nearest neighboring codes
title_short QSPR modeling of Gibbs free energy of organic compounds by weighting of nearest neighboring codes
title_full QSPR modeling of Gibbs free energy of organic compounds by weighting of nearest neighboring codes
title_fullStr QSPR modeling of Gibbs free energy of organic compounds by weighting of nearest neighboring codes
title_full_unstemmed QSPR modeling of Gibbs free energy of organic compounds by weighting of nearest neighboring codes
title_sort qspr modeling of gibbs free energy of organic compounds by weighting of nearest neighboring codes
publishDate 2005
url http://sedici.unlp.edu.ar/handle/10915/133006
work_keys_str_mv AT castroeduardoalberto qsprmodelingofgibbsfreeenergyoforganiccompoundsbyweightingofnearestneighboringcodes
AT toropovaallap qsprmodelingofgibbsfreeenergyoforganiccompoundsbyweightingofnearestneighboringcodes
AT toropovandreya qsprmodelingofgibbsfreeenergyoforganiccompoundsbyweightingofnearestneighboringcodes
AT mukhamedjanovadv qsprmodelingofgibbsfreeenergyoforganiccompoundsbyweightingofnearestneighboringcodes
bdutipo_str Repositorios
_version_ 1764820454670860290