Low temperature irreversibility induced by thermal cycles on two prototypical phase separated manganites

We have studied the effect of irreversibility induced by repeated thermal cycles on the electric transport and magnetization of polycrystalline samples of La0.5Ca0.5MnO3 and La0.325Pr 0.3Ca0.375MnO3. An increase of the resistivity and a decrease of the magnetization at different temperature ranges a...

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Publicado: 2004
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Acceso en línea:https://bibliotecadigital.exactas.uba.ar/collection/paper/document/paper_09258388_v369_n1-2_p74_Sacanell
http://hdl.handle.net/20.500.12110/paper_09258388_v369_n1-2_p74_Sacanell
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spelling paper:paper_09258388_v369_n1-2_p74_Sacanell2023-06-08T15:51:27Z Low temperature irreversibility induced by thermal cycles on two prototypical phase separated manganites Irreversibility Manganites Phase separation Approximation theory Graph theory Ground state Hydrostatic pressure Magnetization Microstructure Phase separation Phase transitions Polycrystalline materials Sampling Thermal cycling Irreversibility Manganites Manganese compounds We have studied the effect of irreversibility induced by repeated thermal cycles on the electric transport and magnetization of polycrystalline samples of La0.5Ca0.5MnO3 and La0.325Pr 0.3Ca0.375MnO3. An increase of the resistivity and a decrease of the magnetization at different temperature ranges after cycling is obtained in the temperature range between 300 and 30K. Both compounds are known to exhibit intrinsic submicrometric coexistence of phases and undergo a sequence of phase transitions related to structural changes. Changes induced by thermal cycling can be partially inhibited by applying magnetic field and hydrostatic pressure. Our results suggest that the growth and coexistence of phases with different structures gives rise to microstructural tracks and strain accommodation, producing the observed irreversibility. Irrespective of the actual ground state of each compound, the effect of thermal cycling is towards an increase of the amount of the insulating phase in both compounds. © 2003 Elsevier B.V. All rights reserved. 2004 https://bibliotecadigital.exactas.uba.ar/collection/paper/document/paper_09258388_v369_n1-2_p74_Sacanell http://hdl.handle.net/20.500.12110/paper_09258388_v369_n1-2_p74_Sacanell
institution Universidad de Buenos Aires
institution_str I-28
repository_str R-134
collection Biblioteca Digital - Facultad de Ciencias Exactas y Naturales (UBA)
topic Irreversibility
Manganites
Phase separation
Approximation theory
Graph theory
Ground state
Hydrostatic pressure
Magnetization
Microstructure
Phase separation
Phase transitions
Polycrystalline materials
Sampling
Thermal cycling
Irreversibility
Manganites
Manganese compounds
spellingShingle Irreversibility
Manganites
Phase separation
Approximation theory
Graph theory
Ground state
Hydrostatic pressure
Magnetization
Microstructure
Phase separation
Phase transitions
Polycrystalline materials
Sampling
Thermal cycling
Irreversibility
Manganites
Manganese compounds
Low temperature irreversibility induced by thermal cycles on two prototypical phase separated manganites
topic_facet Irreversibility
Manganites
Phase separation
Approximation theory
Graph theory
Ground state
Hydrostatic pressure
Magnetization
Microstructure
Phase separation
Phase transitions
Polycrystalline materials
Sampling
Thermal cycling
Irreversibility
Manganites
Manganese compounds
description We have studied the effect of irreversibility induced by repeated thermal cycles on the electric transport and magnetization of polycrystalline samples of La0.5Ca0.5MnO3 and La0.325Pr 0.3Ca0.375MnO3. An increase of the resistivity and a decrease of the magnetization at different temperature ranges after cycling is obtained in the temperature range between 300 and 30K. Both compounds are known to exhibit intrinsic submicrometric coexistence of phases and undergo a sequence of phase transitions related to structural changes. Changes induced by thermal cycling can be partially inhibited by applying magnetic field and hydrostatic pressure. Our results suggest that the growth and coexistence of phases with different structures gives rise to microstructural tracks and strain accommodation, producing the observed irreversibility. Irrespective of the actual ground state of each compound, the effect of thermal cycling is towards an increase of the amount of the insulating phase in both compounds. © 2003 Elsevier B.V. All rights reserved.
title Low temperature irreversibility induced by thermal cycles on two prototypical phase separated manganites
title_short Low temperature irreversibility induced by thermal cycles on two prototypical phase separated manganites
title_full Low temperature irreversibility induced by thermal cycles on two prototypical phase separated manganites
title_fullStr Low temperature irreversibility induced by thermal cycles on two prototypical phase separated manganites
title_full_unstemmed Low temperature irreversibility induced by thermal cycles on two prototypical phase separated manganites
title_sort low temperature irreversibility induced by thermal cycles on two prototypical phase separated manganites
publishDate 2004
url https://bibliotecadigital.exactas.uba.ar/collection/paper/document/paper_09258388_v369_n1-2_p74_Sacanell
http://hdl.handle.net/20.500.12110/paper_09258388_v369_n1-2_p74_Sacanell
_version_ 1768545654412410880