Mesoporous hybrid and nanocomposite thin films. A sol-gel toolbox to create nanoconfined systems with localized chemical properties

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Mesoporous Thin Films (MTF) can be created by combining sol-gel synthesis, template self-assembly and chemical surface modification. A wide palette of inorganic (oxides, phosphates, carbon-based, etc.) and hybrid organic-inorganic frameworks with a variety of composition, pore sizes, and nanoscale,...

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Autores principales:	Soler-Illia, G.J.A.A., Angelomé, P.C., Fuertes, M.C., Calvo, A., Wolosiuk, A., Zelcer, A., Bellino, M.G., Martínez, E.D.
Formato:	JOUR
Materias:	Functional materials Mesoporous films Mesoporous hybrids Nanochemistry Thin films Biological functions Building blockes Carbon-based Chemical surface modification Complex structure Controlled environment Different length scale Mesoporous thin films Mesoscopics Modular synthesis Monodisperse Multiscales Nano chemistry Nano scale Nano-cavities Nano-confined systems Nanocomposite thin films Organic functional groups Organic-inorganic Pore surface Pore system Pore volume Selected examples Sol-gel synthesis Surface feature Chemical modification Chemical properties Functional groups Gels Nanocomposite films Nanocomposites Optical transfer function Pore size Sol-gel process Sol-gels Sols Surfaces Mesoporous materials
Acceso en línea:	http://hdl.handle.net/20.500.12110/paper_09280707_v57_n3_p299_SolerIllia
Aporte de:	Biblioteca Digital - Facultad de Ciencias Exactas y Naturales (UBA) de Universidad de Buenos Aires

id	todo:paper_09280707_v57_n3_p299_SolerIllia
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spelling	todo:paper_09280707_v57_n3_p299_SolerIllia2023-10-03T15:47:18Z Mesoporous hybrid and nanocomposite thin films. A sol-gel toolbox to create nanoconfined systems with localized chemical properties Soler-Illia, G.J.A.A. Angelomé, P.C. Fuertes, M.C. Calvo, A. Wolosiuk, A. Zelcer, A. Bellino, M.G. Martínez, E.D. Functional materials Mesoporous films Mesoporous hybrids Nanochemistry Thin films Biological functions Building blockes Carbon-based Chemical surface modification Complex structure Controlled environment Different length scale Mesoporous films Mesoporous hybrids Mesoporous thin films Mesoscopics Modular synthesis Monodisperse Multiscales Nano chemistry Nano scale Nano-cavities Nano-confined systems Nanocomposite thin films Organic functional groups Organic-inorganic Pore surface Pore system Pore volume Selected examples Sol-gel synthesis Surface feature Chemical modification Chemical properties Functional groups Functional materials Gels Nanocomposite films Nanocomposites Optical transfer function Pore size Sol-gel process Sol-gels Sols Surfaces Thin films Mesoporous materials Mesoporous Thin Films (MTF) can be created by combining sol-gel synthesis, template self-assembly and chemical surface modification. A wide palette of inorganic (oxides, phosphates, carbon-based, etc.) and hybrid organic-inorganic frameworks with a variety of composition, pore sizes, and nanoscale, organic or biological functions located in the inorganic skeleton, pore surface or pore interior can be obtained. The properties of the functional pore systems are tuned by the pore size and geometry, wall composition and surface features. These MTF with interesting electronic and optical controlled features are indeed a "nanofacility". Well-defined monodisperse sized pores also act as nanoreactors, or nanocavities with controlled environment and behaviour. In the last years, the production of accessible MTF, in which either the pore surface or pore volume can be modified by organic functional groups or nanoparticles has been thoroughly explored. Each highly controlled MTF originated from a reproducible and modular synthesis is in itself a building block for more complex structures, presenting order at different length scales (molecular, mesoscopic, macroscopic), and novel properties derived thereof. Selected examples of optical and chemical behaviour of these multiscale materials are presented to illustrate these points. © 2010 Springer Science+Business Media, LLC. Fil:Soler-Illia, G.J.A.A. Universidad de Buenos Aires. Facultad de Ciencias Exactas y Naturales; Argentina. Fil:Angelomé, P.C. Universidad de Buenos Aires. Facultad de Ciencias Exactas y Naturales; Argentina. Fil:Zelcer, A. Universidad de Buenos Aires. Facultad de Ciencias Exactas y Naturales; Argentina. Fil:Bellino, M.G. Universidad de Buenos Aires. Facultad de Ciencias Exactas y Naturales; Argentina. JOUR info:eu-repo/semantics/openAccess http://creativecommons.org/licenses/by/2.5/ar http://hdl.handle.net/20.500.12110/paper_09280707_v57_n3_p299_SolerIllia
institution	Universidad de Buenos Aires
institution_str	I-28
repository_str	R-134
collection	Biblioteca Digital - Facultad de Ciencias Exactas y Naturales (UBA)
topic	Functional materials Mesoporous films Mesoporous hybrids Nanochemistry Thin films Biological functions Building blockes Carbon-based Chemical surface modification Complex structure Controlled environment Different length scale Mesoporous films Mesoporous hybrids Mesoporous thin films Mesoscopics Modular synthesis Monodisperse Multiscales Nano chemistry Nano scale Nano-cavities Nano-confined systems Nanocomposite thin films Organic functional groups Organic-inorganic Pore surface Pore system Pore volume Selected examples Sol-gel synthesis Surface feature Chemical modification Chemical properties Functional groups Functional materials Gels Nanocomposite films Nanocomposites Optical transfer function Pore size Sol-gel process Sol-gels Sols Surfaces Thin films Mesoporous materials
spellingShingle	Functional materials Mesoporous films Mesoporous hybrids Nanochemistry Thin films Biological functions Building blockes Carbon-based Chemical surface modification Complex structure Controlled environment Different length scale Mesoporous films Mesoporous hybrids Mesoporous thin films Mesoscopics Modular synthesis Monodisperse Multiscales Nano chemistry Nano scale Nano-cavities Nano-confined systems Nanocomposite thin films Organic functional groups Organic-inorganic Pore surface Pore system Pore volume Selected examples Sol-gel synthesis Surface feature Chemical modification Chemical properties Functional groups Functional materials Gels Nanocomposite films Nanocomposites Optical transfer function Pore size Sol-gel process Sol-gels Sols Surfaces Thin films Mesoporous materials Soler-Illia, G.J.A.A. Angelomé, P.C. Fuertes, M.C. Calvo, A. Wolosiuk, A. Zelcer, A. Bellino, M.G. Martínez, E.D. Mesoporous hybrid and nanocomposite thin films. A sol-gel toolbox to create nanoconfined systems with localized chemical properties
topic_facet	Functional materials Mesoporous films Mesoporous hybrids Nanochemistry Thin films Biological functions Building blockes Carbon-based Chemical surface modification Complex structure Controlled environment Different length scale Mesoporous films Mesoporous hybrids Mesoporous thin films Mesoscopics Modular synthesis Monodisperse Multiscales Nano chemistry Nano scale Nano-cavities Nano-confined systems Nanocomposite thin films Organic functional groups Organic-inorganic Pore surface Pore system Pore volume Selected examples Sol-gel synthesis Surface feature Chemical modification Chemical properties Functional groups Functional materials Gels Nanocomposite films Nanocomposites Optical transfer function Pore size Sol-gel process Sol-gels Sols Surfaces Thin films Mesoporous materials
description	Mesoporous Thin Films (MTF) can be created by combining sol-gel synthesis, template self-assembly and chemical surface modification. A wide palette of inorganic (oxides, phosphates, carbon-based, etc.) and hybrid organic-inorganic frameworks with a variety of composition, pore sizes, and nanoscale, organic or biological functions located in the inorganic skeleton, pore surface or pore interior can be obtained. The properties of the functional pore systems are tuned by the pore size and geometry, wall composition and surface features. These MTF with interesting electronic and optical controlled features are indeed a "nanofacility". Well-defined monodisperse sized pores also act as nanoreactors, or nanocavities with controlled environment and behaviour. In the last years, the production of accessible MTF, in which either the pore surface or pore volume can be modified by organic functional groups or nanoparticles has been thoroughly explored. Each highly controlled MTF originated from a reproducible and modular synthesis is in itself a building block for more complex structures, presenting order at different length scales (molecular, mesoscopic, macroscopic), and novel properties derived thereof. Selected examples of optical and chemical behaviour of these multiscale materials are presented to illustrate these points. © 2010 Springer Science+Business Media, LLC.
format	JOUR
author	Soler-Illia, G.J.A.A. Angelomé, P.C. Fuertes, M.C. Calvo, A. Wolosiuk, A. Zelcer, A. Bellino, M.G. Martínez, E.D.
author_facet	Soler-Illia, G.J.A.A. Angelomé, P.C. Fuertes, M.C. Calvo, A. Wolosiuk, A. Zelcer, A. Bellino, M.G. Martínez, E.D.
author_sort	Soler-Illia, G.J.A.A.
title	Mesoporous hybrid and nanocomposite thin films. A sol-gel toolbox to create nanoconfined systems with localized chemical properties
title_short	Mesoporous hybrid and nanocomposite thin films. A sol-gel toolbox to create nanoconfined systems with localized chemical properties
title_full	Mesoporous hybrid and nanocomposite thin films. A sol-gel toolbox to create nanoconfined systems with localized chemical properties
title_fullStr	Mesoporous hybrid and nanocomposite thin films. A sol-gel toolbox to create nanoconfined systems with localized chemical properties
title_full_unstemmed	Mesoporous hybrid and nanocomposite thin films. A sol-gel toolbox to create nanoconfined systems with localized chemical properties
title_sort	mesoporous hybrid and nanocomposite thin films. a sol-gel toolbox to create nanoconfined systems with localized chemical properties
url	http://hdl.handle.net/20.500.12110/paper_09280707_v57_n3_p299_SolerIllia
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Mesoporous hybrid and nanocomposite thin films. A sol-gel toolbox to create nanoconfined systems with localized chemical properties

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